Aired: September 10, 1966
The Bubbler kidnaps the Shah of Shish-Ka-Bob and it's up to the Impossibles to rescue him.
Aired: September 10, 1966
Dr. Shock uses his Master Mix Monster Machine to turn his assistant Igor into an electricity-absorbing monster.
Aired: September 10, 1966
The Spinner steals a $1,000,000 tiara.
Aired: September 17, 1966
The Paper Doll Man steals a top secret plan and is out to steal the second part.
Aired: September 17, 1966
Professor Conroy and Buzz unveil the blueprints for the Spy Detector XK-00-7 at a Maximum Security Building. Unfortunately, the blueprints are targeted by the Spyder Man.
Aired: September 17, 1966
Beamatron steals a priceless painting from a ship.
Aired: September 24, 1966
The Burrower uses his burrowing machine to steal half a million dollars from the bank and dig ten miles down to his lair.
Aired: September 24, 1966
Upon an encounter with Buzz at the wax museum, Mr. Menace uses his monsters Godzonka, Gorillis and Cyclaws in an attack upon San Francisco.
Aired: September 24, 1966
Timeatron uses his time cabinet to bring villains from the past to pillage for him.
Aired: October 01, 1966
Smogula freezes the Impossibles and seals them within a cave, so they will not interfere with his plans to conquer Empire City.
Aired: October 01, 1966
A giant alien brain arrives on Earth and captures Buzz and Frankenstein Jr.
Aired: October 01, 1966
The Speck uses a formula to shrink himself in order to photograph top secret plans.
Aired: October 08, 1966
To get the Impossibles out of the way, Fero uses his fiddle to transport them to different planets.
Aired: October 08, 1966
A giant alien brain arrives on Earth and captures Buzz and Frankenstein Jr.
Aired: October 08, 1966
Mother Gruesome invents a machine that brings villainous storybook characters out of their stories to help her with her crimes.
Aired: October 15, 1966
Televisatron transports the Impossibles to different television shows.
Aired: October 15, 1966
The alien Zargon unleashes his warrior Destructo to conquer Earth.
Aired: October 15, 1966
The Dauber uses a special brush where anything he paints becomes real.
Aired: October 22, 1966
Aquator has stolen a secret formula from a scientist who is friends with Big D and shrinks himself to microscopic size in order to get all the microscopic creatures to become large.
Aired: October 22, 1966
Plant Man thaws the last three prehistoric plants (the Carnivorous Chewer, the Creeping Crusher and the Fire-Breathing Snapdragon) from a glacier and then sprays them with his Obedience Ray in a plot to eliminate Buzz and Frankenstein Jr.
Aired: October 22, 1966
Professor Stretch causes havoc with his elastic abilities.
Aired: October 29, 1966
The Dragster has stolen a valuable item.
Aired: October 29, 1966
The Mad Inventor has invented the Double Identity Duplicator Projector to create living images he can control.
Aired: October 29, 1966
The Spinner returns and steals a priceless pooch.
Aired: November 05, 1966
The Surfer takes pictures of a top secret submarine.
Aired: November 05, 1966
The Junk Man creates the Colossal Junk Monster in a plot to eliminate Frankenstein Jr.
Aired: November 05, 1966
Aired: November 12, 1966
Spraysol steals top secret documents.
Aired: November 12, 1966
Buzz and Frankenstein Jr. guard the Navy's new Hydrotomic Submarine to prevent Dr. Hook and his aquatic monsters from stealing it.
Aired: November 12, 1966
The Sculptor turns people into statues.
Aired: November 19, 1966
The Archer steals a priceless violin and a million dollars.
Aired: November 19, 1966
Zorbo the Great creates a genie and plans to use its three wishes in order to defeat Frankenstein Jr. and conquer the world.
Aired: November 19, 1966
The Inflator creates giant balloon monsters to help him commit crimes.
Aired: November 26, 1966
The Diamond Dazzler steals a precious diamond in order to awaken the genie within.
Aired: November 26, 1966
Birdman and his robotic birds Vulturo, Rodantus, and King Condor abduct two astronauts and hold them for a ransom of $1,000,000.
Aired: November 26, 1966
The Paper Doll Man returns and causes trouble.
Aired: December 03, 1966
A witch named Cronella Critch robs a charity for orphans party.
Aired: December 03, 1966
Sertano the Satellite King, an alien from Galaxy X, uses a gravity ray in order to get Earth to surrender. Buzz and Frankenstein Jr. must defeat Sertano's robots in order to defeat him.
Aired: December 03, 1966
The Twister is stealing precious jewels.
Aired: December 10, 1966
Professor Stretch returns and creates a rubber monster to help him.
Aired: December 10, 1966
Aired: December 10, 1966
The Tapper transmits himself over phone lines.
Aired: December 17, 1966
The Angler steals secret space research.
Aired: December 17, 1966
To perform a crime wave in London, Baron Von Ghoul creates robotic versions of the horror movie monsters the Electroflying Firefly, the Menacing Mummy, and the Wicked Werewolf.
Aired: December 17, 1966
The Ringmaster puts on a circus and robs from those who attend.
Aired: December 24, 1966
Billy the Kidder is a cowboy who rides a robotic horse and plans to rob the U.S. Mint.
Aired: December 24, 1966
The Mad Inventor has invented the Monstermobile and uses its many gadgets to commit crimes.
Aired: December 24, 1966
Dr. Futuro comes from the 40th century to the twentieth century to steal a million dollar gold brick.
Aired: December 31, 1966
The Clutcher uses an invention that brings his gloves to life.
Aired: December 31, 1966
Mr. Menace uses his putty monster to steal a $1,000,000 coin collection and even kidnaps Buzz. It is up to Frankenstein Jr. to rescue Buzz and defeat Mr. Menace.
Aired: December 31, 1966
Mr. Instant uses his insta-gun that can make anything in an instant.
Aired: January 07, 1967
The Batter kidnaps a baseball star and holds him for ransom.
Aired: January 07, 1967
Dr. Spectro creates three giant ghoulish ghosts in order to take over Penciltrainia.
Aired: January 07, 1967
Mr. Ice and his henchman Freezer Freezer freeze the city in order to take it over.